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George R Aiken

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Western North America is a region defined by extreme gradients in geomorphology and climate, which support a diverse array of ecological communities and natural resources. The region also has extreme gradients in mercury (Hg) contamination due to a broad distribution of inorganic Hg sources. These diverse Hg sources and a varied landscape create a unique and complex mosaic of ecological risk from Hg impairment associated with differential methylmercury (MeHg) production and bioaccumulation. Understanding the landscape-scale variation in the magnitude and relative importance of processes associated with Hg transport, methylation, and MeHg bioaccumulation requires a multidisciplinary synthesis that transcends small-scale...
Categories: Publication; Types: Citation
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Permafrost (perennially frozen) and active-layer (seasonally thawed) soils varying in soil carbon (C) and nitrogen (N) content and radiocarbon age were collected from three sites in interior Alaska to determine potential release of dissolved organic carbon (DOC), total dissolved N (TDN), dissolved organic nitrogen (DON), and dissolved inorganic nitrogen (DIN) upon thaw. Soil cores were cut into 15 cm thick sections, and deep active-layer (15-30 cm above the permafrost boundary) and shallow permafrost (15-30 cm below the permafrost boundary) sections were thawed and leached with deionized water. Soil leachates were analyzed for DOC, TDN, nitrate (NO3-), and ammonium (NH4+) concentrations, dissolved organic matter...
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Understanding the emissions of mercury (Hg) from wildfires is important for quantifying the global atmospheric Hg sources. Emissions of Hg from soils resulting from wildfires in the Western United States was estimated for the 2000 to 2013 period, and the potential emission of Hg from forest soils was assessed as a function of forest type and soil-heating. Wildfire released an annual average of 3100 ± 1900 kg-Hg y-1 for the years spanning 2000-2013 in the 11 states within the study area. This estimate is nearly 5-fold lower than previous estimates for the study region. Lower emission estimates are attributed to an inclusion of fire severity within burn perimeters. Within reported wildfire perimeters, the average...
Categories: Publication; Types: Citation
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This dataset includes the field measurements and laboratory analyses of surface water, seston, and sediment collected from Lake Powell, within Glen Canyon National Recreation area (GLCA), during high flow (May-June 2014) and low flow (August 2015) conditions. The study area includes 12-13 sampling sites that follow a transect spanning the entire length of the reservoir from the Colorado River inflow to the Glen Canyon dam, as well as the San Juan River arm, the Escalante River arm and West Canyon. Bed sediment samples were analyzed for mercury speciation, methylmercury production and degradation rates, total reduced sulfur, iron speciation, organic content, and 16S rRNA gene templates as a proxy for microbial abundances....
The overall objective of this project is to determine the role of chemical processes associated with dissolved organic carbon (DOC) on the transport and reactivity of both naturally occurring and anthropogenic compounds. Defining the roles of DOC in environmental and geochemical processes is critical to understanding the nature and quality of the Nation’s water resources, and is important for future management of these resources. This field of study has increased in relevancy as numerous environmental problems have been linked to processes involving organic matter. My project attempts to meet these needs by focusing on the chemical mechanisms controlling the fate, transport, and reactivity of naturally occurring...
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