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A combination of cosmogenic and artificial 35S was used to assess the movement of sulfur in a steep Central European catchment affected by spruce die-back. The Jezercaroní catchment, Kruscaronné Hory Mts. (Czech Republic) is characterized by a large disproportion between atmospheric S input and S output via stream discharge, with S output currently exceeding S input three times. A relatively high natural concentration of cosmogenic 35S (42 mBq L-1) was found in atmospheric deposition into the catchment in winter and spring of 2000. In contrast, stream discharge contained only 2 mBq L-1. Consequently, more than 95% of the deposited S is cycled or retained within the catchment for more than several months, while older...